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Volume 124, Issue 17
22 April 2024
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Research Article| April 23 2024
Shuwei Sun;
Shuwei Sun
(Data curation, Formal analysis, Validation, Writing – original draft, Writing – review & editing)
International Joint Research Laboratory of New Energy Materials and Devices of Henan Province, School of Physics and Electronics, Henan University
, Kaifeng 475004,
People's Republic of China
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Ying Bai
Ying Bai a)
(Conceptualization, Data curation, Formal analysis, Funding acquisition, Validation, Writing – review & editing)
International Joint Research Laboratory of New Energy Materials and Devices of Henan Province, School of Physics and Electronics, Henan University
, Kaifeng 475004,
People's Republic of China
a)Author to whom correspondence should be addressed: ybai@henu.edu.cn
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Author & Article Information
a)Author to whom correspondence should be addressed: ybai@henu.edu.cn
Appl. Phys. Lett. 124, 171602 (2024)
Article history
Received:
March 02 2024
Accepted:
April 14 2024
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Citation
Shuwei Sun, Ying Bai; High-entropy layer assisting quasi-zero-strain cathodes for P2-Na2/3Ni1/3Mn2/3O2. Appl. Phys. Lett. 22 April 2024; 124 (17): 171602. https://doi.org/10.1063/5.0206490
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Layered transition metal oxides have attracted much attention for high-energy density sodium ion batteries. However, most P2-type layered oxides undergo a large volume change when they are charged at a deep desodiated state, accompanied by inevitable anisotropic stress, leading to poor structural stability and terrible ion transfer. In this work, a high entropy (HE) material with a robust structure and fast ion transportation was decorated on P2-Na2/3Ni1/3Mn2/3O2 (NM) layered oxides. The unique characteristics of HE shells with similar lattice constants could effectively depress particle crack and exfoliation through buffering severe lattice strains, thus leading to enhanced cycling stability and kinetic properties of the HE-NM electrode. In situ x-ray diffraction analysis confirms that the volume expansion of NM could be prominently restrained both under thermal treatments and electrochemical after HE decoration. The modified cathode exhibits a volume change as low as 0.5%. The findings highlight the significance and superiority of the HE coating layer and provide insight for the rational design of high-performance sodium-ion batteries.
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© 2024 Author(s). Published under an exclusive license by AIP Publishing.
2024
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